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Great Valley is a town that is centrally located in Cattaraugus County, northeast of the city of Salamanca, New York, United States. The population was 1,974 at the 2010 census. The town took its name on its local geographical setting, a relative comparison of two tributaries of the Allegheny River. The Town was formed in 1818, taken from part of the Town of Olean. Great Valley has Zip code 14741.